My all time favourite is Wolf's Rain ^^
http://www.youtube.com/watch?v=Ygxy_...eature=related
Second Favourite i think is School Days. I mean, how many anime do you know where two of the three main characters die in the most epic bad ending ever?
http://www.youtube.com/watch?v=GeCslaQk5_c
and then I also like the following:
FLCL
Mai Hime
Mai Otome (+Mai Otome Zwei and Mai Otome O.Sifr)
Elfen Lied
Serial Experiments Lain
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